Third-order optical response in d-wave altermagnets: Analytical and numerical results from microscopic model

Abstract: Altermagnets represent a novel category of magnetic materials characterized by zero net magnetization yet featuring spin-split band structures, and they demonstrate distinctive orbital-spin locking phenomena. Commencing from the minimal multi-orbital tight-binding Hamiltonian of d-wave altermagnets, we conduct an analysis of the general formulas for the third-order injection and shift currents. These currents are solely determined by the quantum metric and quantum connection, being free from Berry curvature contamination. In the ideal scenario where the $δ$-bond hopping $V_δ$ approaches zero ($V_δ= 0$), we derive closed-form analytical solutions for the third-order photoconductivities. For the general situation with a finite value of $V_δ$, we present a perturbative analytical solution within the limit of $V_δ\ll V_π$, and this solution is verified through numerical calculations. Our research establishes a comprehensive theoretical description of the third-order optospintronic responses in d-wave altermagnets based on a microscopic model. Moreover, it offers a viable approach for the experimental observation of pure quantum geometric effects.